Rose, H J and Jones, G A, 1984, A new kind of natural radioactivity: Nature, v 307, p 245-247.
From a systematic study of the properties of nuclei heavier than lead, we have concluded that, in one or two cases, radioactive decay by emission of a particle heavier than the alpha-particle might be observable in competition with the latter. We have observed such decay in 223Ra which occurs in the natural radioactive series emanating from 235U. Two 'by-pass' modes seem likely: emission of 14C, to 209Pb, with a Q-value of 32 MeV; and of 12C, to 211Pb, with a Q-value of 28 MeV. (Emissions of 13C and 15C from the same nucleus have a priori emission rates similar to that of 12C, but the emission of alpha-like nuclei seems more likely.) In this study we have used a solid-state counter telescope to identify the charge of the particle emitted, and, for greater convenience, a source of 227Ac (half life 21 yr), with which the lower members of the series, including 223Ra, are in secular equilibrium. We have observed particles identifiable as carbon ions and, from their energy and emission rate, they are 14C rather than other carbon isotopes. The branching ratio for emission of 14C nuclei relative to alpha-particles from 223Ra is 8.5 plusminus 2.5x10-10, corresponding to a reduced width (preformation probability) smaller by a factor of approx 10^5 to 10^6.
Your turn, Bob. This is my
third time asking you to answer my question. You told me you'd answer once I posted the journal article supporting my position. That's done now, what will be your excuse this time? Here are the questions again:
Why did you ignore what I just posted? Since you obviously believe carbon dating the "samples" would be of value, don't you feel you have at least some obligation to reason to explain why you are rather unconcerned with the fact that organic solvents were used in the isolation / extraction process? I also like how you failed to mention how exactly they were supposed to scrap together a measurable amount of the substance when the best they could isolate was extremely diffuse scraps.